Wednesday, June 18, 2008
Room 4 (McKimmon Conference Center)
440

Colloid Science and the Solubility Challenges in Developing Intravenous Formulations

Rima Patel, Shahla Jamzad, Ritu Kaushik, Irina Kadiyala, and Rossitza Alargova. Vertex Pharmaceuticals Inc. Cambridge, MA 02139, Cambridge, MA

Development of an intravenous (i.v.) formulation involves: (i) solubilization of the drug on a molecular level (solution) or in the form of nanostructures, (ii) keeping the formulation stable for a certain period of time to allow safe storage and/or administration, and (iii) preventing aggregate formation upon mixing with blood during administration. The success of each step depends on the solution behavior of the drug and the fine balance between the colloidal interactions involved. Therefore, deep understanding of the colloidal behavior is a prerequisite for successful formulation development.

The ideal parenteral formulation should comprise an isotonic solution with pH close to the physiological value of 7.4, and contain only pharmaceutically acceptable ingredients. Meeting these criteria, however, is very often precluded by the low aqueous solubility of the drug. The number of poorly soluble drugs has increased dramatically during the last few decades and resulted in a great variety of parenteral products: in addition to simple solutions, these include microemulsions, emulsions, liposomes, particulate systems, complexes, etc.

When the parent drug is a weak base or acid, the solubility problem can be readily overcome by simple adjustment of the pH to low or high values and salt formation. However, preparing a solution of the drug alone rarely results in a robust formulation as small variations in pH may lead to drug precipitation. In addition, extreme pH values are harmful to patients and might require more complicated ways of administration, such as premixing of stock solutions in the administration set prior to infusion in the body (Y-setup).

The present work describes some of the most common problems related to colloid and interface science when developing an i.v. formulation. The focus is mainly on drugs with extremely low solubility and high melting point (strong crystal lattice). The behavior of both ionizable and nonionizable molecules is examined and analyzed. The paper also presents a critical discussion of each step of the formulation development process, including the in-vitro studies needed to evaluate the formulation behavior in the administration sets.